Aura MLS HCl Depletion and PSC-Induced Areas in the Antarctic. Part 1: 2006, Climate-Chemistry Assessment

      Аннотация: The work presented here evaluated chlorine activation via sulfate aerosol (SA) in the Southern Hemisphere 2006 stratosphere, based on satellite measurements of water vapor (H2O) and constant values of SA, by implementing the TACL formula of [1] in contrast to the TNAT formula of [2]. The results indicated that the former formula was not completely sufficient for accurately modeling areas of depleted HCl and chlorine deactivation for all pressure surfaces in the Antarctic stratosphere. Based on the results of this study, the role of SA in chlorine activation appears to be more important at lower altitudes than for areas higher in the stratosphere.

Ключевые слова: hydrogen chloride, Chlorine activation, Polar Stratospheric Clouds, satellite observations, Antarctic stratosphere, sulfate aerosol